Oral Presentation 6th Modern Solid Phase Peptide Synthesis & Its Applications Symposium 2017

Development of synthetic polymyxins for targeting Gram-negative ‘superbugs’ (#24)

Kade D Roberts 1 , Jiping Wang 1 , Olga Lomovskaya 2 , David C Griffith 2 , Scott J Hecker 2 , Michael N Dudley 2 , Philip E Thompson 1 , Roger L Nation 1 , Tony Velkov 1 , Jian Li 3 4
  1. Monash Institute of Pharmaceutical Sciences, Monash University, Parkville, VIC, Australia
  2. The Medicines Company, San Diego, California, United States of America
  3. Monash Biomedicine Discovery Institute, Monash University, Clayton, Victoria, Australia
  4. Department of Microbiology, Monash University, Clayton, Victoria, Australia

The emergence of multi-drug resistant (MDR) Gram-negative bacterial pathogens such as Pseudomonas aeruginosa, Acinetobacter baumannii and Klebsiella pneumoniae has become a major global health issue. This problem has been further compounded by the lack of development of new antibiotics targeting these Gram-negative bacteria. This has forced clinicians to resort to using ‘old’ antibiotics such as the cyclic lipopeptides, polymyxin B and colistin as last-line therapy against these problematic ‘superbugs’ [1,2]. However, the effective use of these antibiotic peptides in the clinic is significantly hampered by their potential for nephrotoxicity. Recent clinical studies have shown that polymyxin-associated nephrotoxicity can occur in up to 60% of patients when administered intravenously and is the major dose-limiting factor for their optimal use [3,4,5]. This can lead to suboptimal dosing of the polymyxins, which can increase the risk of death and promote polymyxin resistance [6,7].

In this presentation we report on our ongoing pre-clinical polymyxin drug development program, a National Institutes of Health (NIH) funded joint academic-industry collaboration between Monash University and The Medicines Company (USA) [8]. This program aims to produce new polymyxin peptide clinical candidates with improved safety and efficacy over the currently used drugs, polymyxin B and colistin. Aspects of our novel drug design strategy and lead optimization studies will be discussed. To date a number of promising lead candidates have been identified with significantly improved safety profiles and are being progressed towards clinical evaluation.

  1. Velkov T., et al. 2013, Future Microbiol. 8, 711-724.
  2. Nation R. L., et al. 2015, Lancet. Infect. Dis. 15, 225-234.
  3. Kubin C. J., et al. 2012, J. Infect. 65, 80-87.
  4. Akajagbor D. S., et al. 2013, Clin. Infect. Dis. 57, 1300-1303.
  5. Rigatto M. H., et al. 2015, J. Antimicrob. Chemother. 70, 1552-1557.
  6. Onufrak N. J., et al. 2017, Antimicrob Agents Chemother. 61, e00208-17.
  7. Dubrovskaya Y., et al. 2013, Antimicrob Agents Chemother. 57, 5394-5397.
  8. Monash University News, 11 June 2012, Major NIH grant to strike down superbugs